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are reviewed: mononuclear Re(I) complexes, mixed systems with two different Re(I) complexes, and supramolecule systems with a Re(I) complex connected to a ruthenium(II) complex. We focus on the mechanistic studies and the architecture for constructing the photocatalytic systems based on the mechanism.", "publicationTitle": "Coordination Chemistry Reviews", "publisher": "", "place": "", "date": "February 2010", "volume": "254", "issue": "3–4", "section": "", "partNumber": "", "partTitle": "", "pages": "346-354", "series": "Inorganic Reaction MechanismsA Tribute to Ralph Pearson on the occasion of his 90th birthday", "seriesTitle": "", "seriesText": "", "journalAbbreviation": "Coordination Chemistry Reviews", "DOI": "10.1016/j.ccr.2009.09.030", "citationKey": "", "url": "http://www.sciencedirect.com/science/article/pii/S0010854509002501", "accessDate": "2016-04-08T13:33:28Z", "PMID": "", "PMCID": "", "ISSN": "0010-8545", "archive": "", "archiveLocation": "", "shortTitle": "", "language": "", "libraryCatalog": "ScienceDirect", "callNumber": "", "rights": "", "extra": "", "tags": [ { "tag": "CO2 reduction", "type": 1 }, { "tag": "Photocatalyst", "type": 1 }, { "tag": "Rhenium complex", "type": 1 }, { "tag": "Ruthenium complex", "type": 1 }, { "tag": "Supramolecule", "type": 1 } ], "collections": [ "X89VJ8JA" ], "relations": {}, "dateAdded": "2016-04-08T13:33:28Z", "dateModified": "2016-04-08T13:33:28Z" } }, { "key": "UBPJF764", "version": 63, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/UBPJF764", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/UBPJF764", "type": "text/html" }, "up": { "href": "https://api.zotero.org/groups/399754/items/FV6MHWN8", "type": "application/json" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } } }, "data": { "key": "UBPJF764", "version": 63, "parentItem": "FV6MHWN8", "itemType": "attachment", "linkMode": "imported_url", "title": "Snapshot", "accessDate": "2016-04-08T13:27:24Z", "url": "http://pubs.rsc.org/en/Content/ArticleLanding/2013/EE/c3ee41272e#!divAbstract", "note": "", "contentType": "text/html", "charset": "utf-8", "filename": "c3ee41272e.html", "md5": "773b4c6351807305e3d16511ae5c059e", "mtime": 1460122044909, "tags": [], "relations": {}, "dateAdded": "2016-04-08T13:27:24Z", "dateModified": "2016-04-08T13:27:24Z" } }, { "key": "FV6MHWN8", "version": 62, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/FV6MHWN8", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/FV6MHWN8", "type": "text/html" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } }, "creatorSummary": "Kondratenko et al.", "parsedDate": "2013-10-18", "numChildren": 1 }, "data": { "key": "FV6MHWN8", "version": 62, "itemType": "journalArticle", "title": "Status and perspectives of CO2 conversion into fuels and chemicals by catalytic, photocatalytic and electrocatalytic processes", "creators": [ { "creatorType": "author", "firstName": "Evgenii V.", "lastName": "Kondratenko" }, { "creatorType": "author", "firstName": "Guido", "lastName": "Mul" }, { "creatorType": "author", "firstName": "Jonas", "lastName": "Baltrusaitis" }, { "creatorType": "author", "firstName": "Gastón O.", "lastName": "Larrazábal" }, { "creatorType": "author", "firstName": "Javier", "lastName": "Pérez-Ramírez" } ], "abstractNote": "This review highlights recent developments and future perspectives in carbon dioxide usage for the sustainable production of energy and chemicals and to reduce global warming. We discuss the heterogeneously catalysed hydrogenation, as well as the photocatalytic and electrocatalytic conversion of CO2 to hydrocarbons or oxygenates. Various sources of hydrogen are also reviewed in terms of their CO2 neutrality. Technologies have been developed for large-scale CO2 hydrogenation to methanol or methane. Their industrial application is, however, limited by the high price of renewable hydrogen and the availability of large-volume sources of pure CO2. With regard to the direct electrocatalytic reduction of CO2 to value-added chemicals, substantial advances in electrodes, electrolyte, and reactor design are still required to permit the development of commercial processes. Therefore, in this review particular attention is paid to (i) the design of metal electrodes to improve their performance and (ii) recent developments of alternative approaches such as the application of ionic liquids as electrolytes and of microorganisms as co-catalysts. The most significant improvements both in catalyst and reactor design are needed for the photocatalytic functionalisation of CO2 to become a viable technology that can help in the usage of CO2 as a feedstock for the production of energy and chemicals. Apart from technological aspects and catalytic performance, we also discuss fundamental strategies for the rational design of materials for effective transformations of CO2 to value-added chemicals with the help of H2, electricity and/or light.", "publicationTitle": "Energy & Environmental Science", "publisher": "", "place": "", "date": "2013-10-18", "volume": "6", "issue": "11", "section": "", "partNumber": "", "partTitle": "", "pages": "3112-3135", "series": "", "seriesTitle": "", "seriesText": "", "journalAbbreviation": "Energy Environ. Sci.", "DOI": "10.1039/C3EE41272E", "citationKey": "", "url": "http://pubs.rsc.org/en/content/articlelanding/2013/ee/c3ee41272e", "accessDate": "2016-04-08T13:27:19Z", "PMID": "", "PMCID": "", "ISSN": "1754-5706", "archive": "", "archiveLocation": "", "shortTitle": "", "language": "en", "libraryCatalog": "pubs.rsc.org", "callNumber": "", "rights": "", "extra": "", "tags": [], "collections": [ "X89VJ8JA" ], "relations": {}, "dateAdded": "2016-04-08T13:27:19Z", "dateModified": "2016-04-08T13:27:19Z" } }, { "key": "PUKIKID5", "version": 61, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/PUKIKID5", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/PUKIKID5", "type": "text/html" }, "up": { "href": "https://api.zotero.org/groups/399754/items/HW2F5GJ6", "type": "application/json" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } } }, "data": { "key": "PUKIKID5", "version": 61, "parentItem": "HW2F5GJ6", "itemType": "attachment", "linkMode": "imported_url", "title": "ACS Full Text Snapshot", "accessDate": "2016-04-08T13:18:09Z", "url": "http://pubs.acs.org/doi/full/10.1021/ja101318k", "note": "", "contentType": "text/html", "charset": "utf-8", "filename": "ja101318k.html", "md5": "78d6fa41a2a1efe7416edb4866ff8a04", "mtime": 1460121491717, "tags": [], "relations": {}, "dateAdded": "2016-04-08T13:18:09Z", "dateModified": "2016-04-08T13:18:09Z" } }, { "key": "J44SQ8H3", "version": 61, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/J44SQ8H3", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/J44SQ8H3", "type": "text/html" }, "up": { "href": "https://api.zotero.org/groups/399754/items/HW2F5GJ6", "type": "application/json" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } }, "numChildren": 0 }, "data": { "key": "J44SQ8H3", "version": 61, "parentItem": "HW2F5GJ6", "itemType": "attachment", "linkMode": "imported_url", "title": "ACS Full Text PDF w/ Links", "accessDate": "2016-04-08T13:18:06Z", "url": "http://pubs.acs.org/doi/pdfplus/10.1021/ja101318k", "note": "", "contentType": "application/pdf", "charset": "", "filename": "Yang et al. - 2010 - Artificial Photosynthesis over Crystalline TiO2-Ba.pdf", "md5": "7e7cf0fc2e213a163ad21c885435344a", "mtime": 1460121487885, "tags": [], "relations": {}, "dateAdded": "2016-04-08T13:18:06Z", "dateModified": "2016-04-08T13:18:08Z" } }, { "key": "HW2F5GJ6", "version": 60, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/HW2F5GJ6", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/HW2F5GJ6", "type": "text/html" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } }, "creatorSummary": "Yang et al.", "parsedDate": "2010-06-23", "numChildren": 2 }, "data": { "key": "HW2F5GJ6", "version": 60, "itemType": "journalArticle", "title": "Artificial Photosynthesis over Crystalline TiO2-Based Catalysts: Fact or Fiction?", "creators": [ { "creatorType": "author", "firstName": "Chieh-Chao", "lastName": "Yang" }, { "creatorType": "author", "firstName": "Yi-Hui", "lastName": "Yu" }, { "creatorType": "author", "firstName": "Bart", "lastName": "van der Linden" }, { "creatorType": "author", "firstName": "Jeffrey C. S.", "lastName": "Wu" }, { "creatorType": "author", "firstName": "Guido", "lastName": "Mul" } ], "abstractNote": "The mechanism of photocatalytic conversion of CO2 and H2O over copper oxide promoted titania, Cu(I)/TiO2, was investigated by means of in situ DRIFT spectroscopy in combination with isotopically labeled 13CO2. In addition to small amounts of 13CO, 12CO was demonstrated to be the primary product of the reaction by the 2115 cm?1 Cu(I)?CO signature, indicating that carbon residues on the catalyst surface are involved in reactions with predominantly photocatalytically activated surface adsorbed water. This was confirmed by prolonged exposure of the catalyst to light and water vapor, which significantly reduced the amount of CO formed in a subsequent experiment in the DRIFT cell. In addition, formation of carboxylates and (bi)carbonates was observed by exposure of the Cu(I)/TiO2 surface to CO2 in the dark. These carboxylates and (bi)carbonates decompose upon light irradiation, yielding predominantly CO2. At the same time a novel carbonate species is produced (having a main absorption at ?1395 cm?1) by adsorption of photocatalytically produced CO on the Cu(I)/TiO2 surface, most likely through a reverse Boudouard reaction of photocatalytically activated CO2 with carbon residues. The finding that carbon residues are involved in photocatalytic water activation and CO2 reduction might have important implications for the rates of artificial photosynthesis reported in many studies in the literature, in particular those using photoactive materials synthesized with carbon containing precursors.", "publicationTitle": "Journal of the American Chemical Society", "publisher": "", "place": "", "date": "June 23, 2010", "volume": "132", "issue": "24", "section": "", "partNumber": "", "partTitle": "", "pages": "8398-8406", "series": "", "seriesTitle": "", "seriesText": "", "journalAbbreviation": "J. Am. Chem. Soc.", "DOI": "10.1021/ja101318k", "citationKey": "", "url": "http://dx.doi.org/10.1021/ja101318k", "accessDate": "2016-04-08T13:18:06Z", "PMID": "", "PMCID": "", "ISSN": "0002-7863", "archive": "", "archiveLocation": "", "shortTitle": "Artificial Photosynthesis over Crystalline TiO2-Based Catalysts", "language": "", "libraryCatalog": "ACS Publications", "callNumber": "", "rights": "", "extra": "", "tags": [], "collections": [ "X89VJ8JA" ], "relations": {}, "dateAdded": "2016-04-08T13:18:06Z", "dateModified": "2016-04-08T13:18:06Z" } }, { "key": "54WE4XMM", "version": 59, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/54WE4XMM", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/54WE4XMM", "type": "text/html" }, "up": { 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Hydrogenation of CO2 to Formic Acid with.pdf", "md5": "cf247304743dfcddb700e813b25c7282", "mtime": 1460119169504, "tags": [], "relations": {}, "dateAdded": "2016-04-08T12:39:19Z", "dateModified": "2016-04-08T12:39:29Z" } }, { "key": "V6VEHN5S", "version": 58, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/V6VEHN5S", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/V6VEHN5S", "type": "text/html" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } }, "creatorSummary": "Xu et al.", "parsedDate": "2013-07-01", "numChildren": 2 }, "data": { "key": "V6VEHN5S", "version": 58, "itemType": "journalArticle", "title": "Catalytic Hydrogenation of CO2 to Formic Acid with Silica-Tethered Iridium Catalysts", "creators": [ { "creatorType": "author", "firstName": "Zheng", "lastName": "Xu" }, { "creatorType": "author", "firstName": "Nicholas D.", "lastName": "McNamara" }, { "creatorType": "author", "firstName": "Gregory T.", "lastName": "Neumann" }, { "creatorType": "author", "firstName": "William F.", "lastName": "Schneider" }, { "creatorType": "author", "firstName": "Jason C.", "lastName": "Hicks" } ], "abstractNote": "", "publicationTitle": "ChemCatChem", "publisher": "", "place": "", "date": "July 1, 2013", "volume": "5", "issue": "7", "section": "", "partNumber": "", "partTitle": "", "pages": "1769-1771", "series": "", "seriesTitle": "", "seriesText": "", "journalAbbreviation": "ChemCatChem", "DOI": "10.1002/cctc.201200839", "citationKey": "", "url": "http://onlinelibrary.wiley.com/doi/10.1002/cctc.201200839/abstract", "accessDate": "2016-04-08T12:39:19Z", "PMID": "", "PMCID": "", "ISSN": "1867-3899", "archive": "", "archiveLocation": "", "shortTitle": "", "language": "en", "libraryCatalog": "Wiley Online Library", "callNumber": "", "rights": "", "extra": "", "tags": [ { "tag": "carbon dioxide", "type": 1 }, { "tag": "hydrogenation", "type": 1 }, { "tag": "iridium", "type": 1 }, { "tag": "organic–inorganic hybrid composites", "type": 1 }, { "tag": "supported catalysts", "type": 1 } ], "collections": [ "X89VJ8JA" ], "relations": {}, "dateAdded": "2016-04-08T12:39:19Z", "dateModified": "2016-04-08T12:39:19Z" } }, { "key": "SK3FG5JM", "version": 57, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/SK3FG5JM", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/SK3FG5JM", "type": "text/html" }, "up": { "href": "https://api.zotero.org/groups/399754/items/GQ6PU23Q", "type": "application/json" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } } }, "data": { "key": "SK3FG5JM", "version": 57, "parentItem": "GQ6PU23Q", "itemType": "attachment", "linkMode": "imported_url", "title": "ScienceDirect Snapshot", "accessDate": "2016-04-08T06:47:03Z", "url": "http://www.sciencedirect.com/science/article/pii/S0021951709002231", "note": "", "contentType": "text/html", "charset": "utf-8", "filename": "S0021951709002231.html", "md5": "34700455c637f532ba4c141783e97abb", "mtime": 1460098023970, "tags": [], "relations": {}, "dateAdded": "2016-04-08T06:47:03Z", "dateModified": "2016-04-08T06:47:03Z" } }, { "key": "GQ6PU23Q", "version": 56, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/GQ6PU23Q", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/GQ6PU23Q", "type": "text/html" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } }, "creatorSummary": "Yan et al.", "parsedDate": "2009-09-10", "numChildren": 1 }, "data": { "key": "GQ6PU23Q", "version": 56, "itemType": "journalArticle", "title": "Visible-light-driven hydrogen production with extremely high quantum efficiency on Pt–PdS/CdS photocatalyst", "creators": [ { "creatorType": "author", "firstName": "Hongjian", "lastName": "Yan" }, { "creatorType": "author", "firstName": "Jinhui", "lastName": "Yang" }, { "creatorType": "author", "firstName": "Guijun", "lastName": "Ma" }, { "creatorType": "author", "firstName": "Guopeng", "lastName": "Wu" }, { "creatorType": "author", "firstName": "Xu", "lastName": "Zong" }, { "creatorType": "author", "firstName": "Zhibin", "lastName": "Lei" }, { "creatorType": "author", "firstName": "Jingying", "lastName": "Shi" }, { "creatorType": "author", "firstName": "Can", "lastName": "Li" } ], "abstractNote": "To efficiently convert solar energy into chemical energy by artificial photosynthesis, we need to develop visible-light-responsive photocatalysts with a high quantum efficiency (QE). Here we report that an artificial photocatalyst (Pt–PdS/CdS) can achieve a QE up to 93% in photocatalytic H2 production in the presence of sacrificial reagents under visible light irradiation, and is very stable under the photocatalytic reaction conditions. The extremely high QE could be achieved by loading as low as 0.30 wt% of Pt and 0.13 wt% of PdS as cocatalysts on CdS.", "publicationTitle": "Journal of Catalysis", "publisher": "", "place": "", "date": "September 10, 2009", "volume": "266", "issue": "2", "section": "", "partNumber": "", "partTitle": "", "pages": "165-168", "series": "", "seriesTitle": "", "seriesText": "", "journalAbbreviation": "Journal of Catalysis", "DOI": "10.1016/j.jcat.2009.06.024", "citationKey": "", "url": "http://www.sciencedirect.com/science/article/pii/S0021951709002231", "accessDate": "2016-04-08T06:46:58Z", "PMID": "", "PMCID": "", "ISSN": "0021-9517", "archive": "", "archiveLocation": "", "shortTitle": "", "language": "", "libraryCatalog": "ScienceDirect", "callNumber": "", "rights": "", "extra": "", "tags": [ { "tag": "Cadmium sulfide", "type": 1 }, { "tag": "Cocatalyst", "type": 1 }, { "tag": "Hydrogen", "type": 1 }, { "tag": "Photocatalysis", "type": 1 }, { "tag": "Quantum efficiency", "type": 1 } ], "collections": [ "X89VJ8JA" ], "relations": {}, "dateAdded": "2016-04-08T06:46:58Z", "dateModified": "2016-04-08T06:46:58Z" } }, { "key": "5MWQRUDF", "version": 55, "library": { "type": "group", "id": 399754, "name": "thinkdifferent1984", "links": { "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984", "type": "text/html" } } }, "links": { "self": { "href": "https://api.zotero.org/groups/399754/items/5MWQRUDF", "type": "application/json" }, "alternate": { "href": "https://www.zotero.org/groups/thinkdifferent1984/items/5MWQRUDF", "type": "text/html" }, "up": { "href": "https://api.zotero.org/groups/399754/items/W7GWEC4B", "type": "application/json" } }, "meta": { "createdByUser": { "id": 2625460, "username": "thomasr1993", "name": "", "links": { "alternate": { "href": "https://www.zotero.org/thomasr1993", "type": "text/html" } } } }, "data": { "key": "5MWQRUDF", "version": 55, "parentItem": "W7GWEC4B", "itemType": "attachment", "linkMode": "imported_url", "title": "ACS Full Text Snapshot", "accessDate": "2016-04-08T06:45:04Z", "url": "http://pubs.acs.org/doi/full/10.1021/ja027751g", "note": "", "contentType": "text/html", "charset": "utf-8", "filename": "ja027751g.html", "md5": "f105ae1f27ef3fdb1bab2695585ef9ed", "mtime": 1460097905616, "tags": [], "relations": {}, "dateAdded": "2016-04-08T06:45:04Z", "dateModified": "2016-04-08T06:45:04Z" } } ]