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            "title": "Global and target analysis of time-resolved spectra",
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                {
                    "creatorType": "author",
                    "firstName": "Ivo H.M.",
                    "lastName": "van Stokkum"
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            "abstractNote": "In (bio)physical/(bio)chemical research the response of a complex system to an externally applied perturbation is often studied. In most cases the obtained response is of a complexity that prohibits direct interpretation of the obtained data. In the case of time-resolved spectroscopy, measurements at multiple wavelengths can often be used to disentangle complex kinetics. These time-resolved spectra can be considered as an example of multiway data. In these lectures, the methodology for global and target analysis of time-resolved spectra is explained, both from a practical, and from a fundamental/mathematical point of view. To fully extract the information from the overwhelming amount of data a model-based analysis is mandatory. This analysis is based upon assumptions regarding the measurement process and upon a physicochemical model for the complex system. The model is composed of building blocks representing scientific knowledge and assumptions, such as the instrument response function, the components of the system connected in a kinetic scheme, and additional properties of the components (e.g. anisotropy). The use of a combined model for the kinetics and for the spectra of the components results in a more powerful spectro-temporal model. The model parameters, like rate constants and spectra, can be estimated from the data, thus providing a concise description of the complex system dynamics. This spectro-temporal modelling approach is illustrated with several case studies.",
            "type": "",
            "date": "2005",
            "publisher": "VU University Amsterdam",
            "place": "",
            "DOI": "",
            "citationKey": "",
            "url": "http://www.nat.vu.nl/~ivo/lecturenotes.pdf",
            "accessDate": "2010-11-17",
            "archive": "",
            "archiveLocation": "",
            "shortTitle": "",
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            "callNumber": "0091",
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            "dateAdded": "2010-11-17T14:12:38Z",
            "dateModified": "2011-10-02T07:31:07Z"
        }
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